Sadly not I'm afraid, in fact for someone who collects game soundtracks, I have none from audo games weerdly.
Personally, i'd say the single most inappropriate game soundtracks I've heard are for the first two donkey Kong country games, ---- released in the mid nineties on the snes.
You'd expect the soundtracks to games where your playing a big ape jumping through levels and climbing ropes mario style to retreave his banana hoard from a bunch of crocodiles to be cutesey, ---- or at least light hearted the way music to most of the Mario, james pond or sonic games was.
nothing like it!
Dk 1 and 2 have some of the best most atmospheric epic game music I've ever heard, in a variety of styles from creepy, to eletronica, to full on semi-orchestral pyratical doom!
Even the last boss to Dk1 had comical music which start out like a merry sea jig (your fighting him on board his pyrate ship), then suddenly becomes a full on semi wrock techno epic mix! --- amusingly enough the bosses own tactics also change, being easy at the start then amazingly difficult later on.
The third game in the series has a few good tracks, but I didn't personally feel it came close to the atmosphere of the first two.
I'd strongly recommend getting these though they're some of my favourites.
Unfortunately, I only have them in spc snes format. You can however download all the soundtracks (along with many more), and a very efficient winamp plugin to play them Here on the snes amp site
There's also an mp3 convertion tool should you want it, but personally I just use the winamp plugin, ---- especially sinse winamp is my music playing program of choice anyway.
With our dreaming and singing, Ceaseless and sorrowless we! The glory about us clinging Of the glorious futures we see,
Our souls with high music ringing; O men! It must ever be
That we dwell in our dreaming and singing, A little apart from ye. (Arthur O'Shaughnessy 1873.)